How can I delete, organize then sync pictures across all devices?

[Windows Central Question]

I am using desktop and laptop PCs, a Lumia phone and Surface Pro 4 tablet. I am using One Drive but apparently not correctly because every attempt to delete the pictures I don't want, organize the ones I do want and get them to show up the same on One Drive across all my devices fails. I just spent and hour in the One Drive folder on my laptop cleaning things up and organizing them, go to my phone and Surface and nothing has changed.

What do I need to do to get everything showing the same in One Drive across my devices? Everything is Windows except the phone which is 8.1 and I am logging in to every device with the same Microsoft account.